Based on the theory of coherence, the model of multi-Gaussian Schell-model(MGSM) beams carrying an edge dislocation generated by the MGSM source is introduced. The analytical cross-spectral density of MGSM beams carry...Based on the theory of coherence, the model of multi-Gaussian Schell-model(MGSM) beams carrying an edge dislocation generated by the MGSM source is introduced. The analytical cross-spectral density of MGSM beams carrying an edge dislocation propagating in oceanic turbulence is derived, and used to study the evolution properties of the MGSM beams carrying an edge dislocation. The results indicate that the MGSM beam carrying an edge dislocation propagating in oceanic turbulence will evolve from the profile with two intensity peaks into a flat-topped beam caused by the MGSM source, and the beam will evolve into the Gaussian-like beam due to the influences of oceanic turbulence in the far field.As the propagation distance increases, the MGSM beam carrying an edge dislocation propagating in oceanic turbulence with the larger rate of dissipation of mean-squared temperature(χT) and ratio of temperature to salinity contribution to the refractive index spectrum(?) or the smaller rate of dissipation of kinetic energy per unit mass of fluid(ε) evolves into the flat-topped beam or a Gaussian beam faster.展开更多
The influence of a high-intensity laser field on the inelastic interactions between a swift B_(3)^(+) cluster ion and a plasma target is studied by means of the linearized Vlasov–Poisson theory.Excitations of the pla...The influence of a high-intensity laser field on the inelastic interactions between a swift B_(3)^(+) cluster ion and a plasma target is studied by means of the linearized Vlasov–Poisson theory.Excitations of the plasma are described by the classical plasma dielectric function.In the presence of the laser field,the general expressions for the induced potential in the target and the interaction force among the ions within the cluster are derived.Based on the numerical solution of the equations of motion for the constituent ions,the Coulomb explosion patterns and the cluster's energy losses are discussed for a range of laser parameters.展开更多
Linear and nonlinear photophysical properties of two novel dipolar compounds named as trans- dimethyl-4-[4＇-（N,N-dimethylamino）-styry1]-pyridin-2,6-dicarboxylate （Xiao-1） and trans-dimethyl-4-[4＇-（N,N-diphenyla...Linear and nonlinear photophysical properties of two novel dipolar compounds named as trans- dimethyl-4-[4＇-（N,N-dimethylamino）-styry1]-pyridin-2,6-dicarboxylate （Xiao-1） and trans-dimethyl-4-[4＇-（N,N-diphenylamino）-styry1]-pyridin-2,6-dicarboxylate （Xiao-2） are investigated by steady-state absorption and fluorescence spectroscopy, Z-scan and two-photon excited fluorescence measurements. Strong two-photon fluorescence emission and the pronounced positive solvatochromism are observed from two compounds. The two-photon absorption cross section of Xiao-2 is about 1.5 times larger than that of Xiao-1. One-color and two-color femtosecond pump-probe experiments are employed to investigate the excited state dynamics of two compounds. The relaxation lifetime of the intra-molecular charge transfer state is determined to be in the hundreds of picosecond domain for both the compounds in THF, and several tens of picosecond in DMSO solutions.展开更多
Ultrafast third-order nonlinear optical response of bulk 6H-SiC undoped and doped with different nitrogen concentrations are investigated utilizing femtosecond Z-scan and optical Kerr effect （OKE） techniques at the ...Ultrafast third-order nonlinear optical response of bulk 6H-SiC undoped and doped with different nitrogen concentrations are investigated utilizing femtosecond Z-scan and optical Kerr effect （OKE） techniques at the wavelength of 800hm. The Z-scan measurement shows that the third-order nonlinear optical susceptibilities of the doped samples are improved in comparison to the intrinsic sample. The OKE results additionally reveal that the instantaneous nonlinear optical response of the samples can be ascribed to the distortion of the electron cloud. The ultrafast transient spectroscopic measurements with the one-color and two-color pump-probe techniques demonstrate that the ultrafast recovery process in subpicosecond domain is induced by two-photon absorption process, while the slow relaxation component reflects the carrier dynamics of the excited electrons.展开更多
The two-photon fluorescence properties and ultrafast responses of a hyperbranched polyyne （hb-DPP-J2） with triphenylamine as the central core, Diketo-Pyrrolo-Pyrrole as the connecting unit and electron acceptor are ...The two-photon fluorescence properties and ultrafast responses of a hyperbranched polyyne （hb-DPP-J2） with triphenylamine as the central core, Diketo-Pyrrolo-Pyrrole as the connecting unit and electron acceptor are studied. The polymer has a D-π-A-π-D conjugated structure along the extended polyyne w-bridge systems, and the effective condugated unit repeats itself in the whole hyperbranehed polymer chain. The polymer exhibits a large two-photon absorption cross section and high fluorescence quantum yields. The ultrafast dynamic results give a deep understanding of the excited energy transfer processes under excitation, and reveal a long relaxation lifetime of the intramolecular charge transfer （ICT） state.展开更多
基金Project supported by the National Natural Science Foundation of China(Grant Nos.11604038,11875096,and 11404048)the Fundamental Research Funds for the Central Universities,China(Grant Nos.3132019182 and 3132019184)
文摘Based on the theory of coherence, the model of multi-Gaussian Schell-model(MGSM) beams carrying an edge dislocation generated by the MGSM source is introduced. The analytical cross-spectral density of MGSM beams carrying an edge dislocation propagating in oceanic turbulence is derived, and used to study the evolution properties of the MGSM beams carrying an edge dislocation. The results indicate that the MGSM beam carrying an edge dislocation propagating in oceanic turbulence will evolve from the profile with two intensity peaks into a flat-topped beam caused by the MGSM source, and the beam will evolve into the Gaussian-like beam due to the influences of oceanic turbulence in the far field.As the propagation distance increases, the MGSM beam carrying an edge dislocation propagating in oceanic turbulence with the larger rate of dissipation of mean-squared temperature(χT) and ratio of temperature to salinity contribution to the refractive index spectrum(?) or the smaller rate of dissipation of kinetic energy per unit mass of fluid(ε) evolves into the flat-topped beam or a Gaussian beam faster.
基金Supported by the National Natural Science Foundation of China under Grant Nos 10705007,11005025,11105022the Doctorial Start-up Foundation of Liaoning Province in China under Grant No 20071067+1 种基金the Fundamental Research Funds for the Central Universities under Grant No 2012TD018the Natural Scientific Research Innovation Foundation in Harbin Institute of Technology under Grant No HIT.NSRIF.2009044.
文摘The influence of a high-intensity laser field on the inelastic interactions between a swift B_(3)^(+) cluster ion and a plasma target is studied by means of the linearized Vlasov–Poisson theory.Excitations of the plasma are described by the classical plasma dielectric function.In the presence of the laser field,the general expressions for the induced potential in the target and the interaction force among the ions within the cluster are derived.Based on the numerical solution of the equations of motion for the constituent ions,the Coulomb explosion patterns and the cluster's energy losses are discussed for a range of laser parameters.
基金supported by the National Natural Science Foundation of China (60978055,10674031,20676034,20876046)Key Project of the Ministry of Education of China (309013)+1 种基金Shanghai Municipal Educational Commission for the Shuguang Fellowship,China (08GG10)Shanghai Eastern Scholarship,China~~
基金Supported by the National Natural Science Foundation of China under Grant Nos 10674031 and 60978055, the Innovation Program of Shanghai Municipal Education Commission （No 09YZ160）, and Shanghai Normal University （No SK200839）.
文摘Linear and nonlinear photophysical properties of two novel dipolar compounds named as trans- dimethyl-4-[4＇-（N,N-dimethylamino）-styry1]-pyridin-2,6-dicarboxylate （Xiao-1） and trans-dimethyl-4-[4＇-（N,N-diphenylamino）-styry1]-pyridin-2,6-dicarboxylate （Xiao-2） are investigated by steady-state absorption and fluorescence spectroscopy, Z-scan and two-photon excited fluorescence measurements. Strong two-photon fluorescence emission and the pronounced positive solvatochromism are observed from two compounds. The two-photon absorption cross section of Xiao-2 is about 1.5 times larger than that of Xiao-1. One-color and two-color femtosecond pump-probe experiments are employed to investigate the excited state dynamics of two compounds. The relaxation lifetime of the intra-molecular charge transfer state is determined to be in the hundreds of picosecond domain for both the compounds in THF, and several tens of picosecond in DMSO solutions.
基金Supported by the National Natural Science Foundation of China under Grant Nos 10674031 and 60978055, the National Taiwan University under Grant Nos NSC-97-2221-E-002-026 and NSC-98-2221-E-002-015-MY3, and the NSF of USA through the Center of Physics and Chemistry of Materials under Grant No HRD-0420516.
文摘Ultrafast third-order nonlinear optical response of bulk 6H-SiC undoped and doped with different nitrogen concentrations are investigated utilizing femtosecond Z-scan and optical Kerr effect （OKE） techniques at the wavelength of 800hm. The Z-scan measurement shows that the third-order nonlinear optical susceptibilities of the doped samples are improved in comparison to the intrinsic sample. The OKE results additionally reveal that the instantaneous nonlinear optical response of the samples can be ascribed to the distortion of the electron cloud. The ultrafast transient spectroscopic measurements with the one-color and two-color pump-probe techniques demonstrate that the ultrafast recovery process in subpicosecond domain is induced by two-photon absorption process, while the slow relaxation component reflects the carrier dynamics of the excited electrons.
基金Supported by the National Natural Science Foundation of China under Grant Nos 11404048,61205154 and 11375034the Fundamental Research Funds for the Central Universities under Grant Nos 3132015233,3132013104,3132014337,3132015144 and3132015152+1 种基金the State Key Laboratory of Fine Chemicals(KF1409)the Program for Liaoning Excellent Talents in University under Grant No LJQ2014051
文摘The two-photon fluorescence properties and ultrafast responses of a hyperbranched polyyne （hb-DPP-J2） with triphenylamine as the central core, Diketo-Pyrrolo-Pyrrole as the connecting unit and electron acceptor are studied. The polymer has a D-π-A-π-D conjugated structure along the extended polyyne w-bridge systems, and the effective condugated unit repeats itself in the whole hyperbranehed polymer chain. The polymer exhibits a large two-photon absorption cross section and high fluorescence quantum yields. The ultrafast dynamic results give a deep understanding of the excited energy transfer processes under excitation, and reveal a long relaxation lifetime of the intramolecular charge transfer （ICT） state.
