Smart electronic textiles with electronic functions like displaying can provide transformative opportunities for wearable devices that traditional rigid devices are hard to realize.A general strategy of enabling texti...Smart electronic textiles with electronic functions like displaying can provide transformative opportunities for wearable devices that traditional rigid devices are hard to realize.A general strategy of enabling textiles to display is weaving light-emitting fibers into textiles and designing control circuits.However,it remains challenging for the current electronic textiles to display full-color images and videos.Here,we demonstrate a large-area integrated electronic textile system(with a size of 72 cm×50 cm)by weaving light-emitting diode(LED)fibers,touch-sensing fibers and polyester fibers,which could display full-color images(with a gamut of 117.6%NTSC)and continuous videos(with a refresh rate of 11.7 Hz)by designing low-voltage supply mode and parallelly transmitting circuits.After integration of touch-sensing fibers,such textile system could achieve various touch display and interactive functions like smart phones or computers,including hand input of text,hand painting,computing and playing games.The stability and durability of textile system withstanding 5000 bending cycles was also demonstrated for wearable applications.The integrated electronic textile system shows similar flexibility and breathability with regular textiles,which is promising to serve as new human-machine interface to change the way in which people interact with electronics.展开更多
水系金属空气电池具有理论能量密度高、安全性高等优点,但受限于金属阳极(如锌、铁、铝、镁)的电化学不可逆性以及碱性电解质对大气中二氧化碳的化学不稳定性.本工作首次设计了一种可充电的铋-空气电池,该电池使用了非碱性的三氟甲磺酸...水系金属空气电池具有理论能量密度高、安全性高等优点,但受限于金属阳极(如锌、铁、铝、镁)的电化学不可逆性以及碱性电解质对大气中二氧化碳的化学不稳定性.本工作首次设计了一种可充电的铋-空气电池,该电池使用了非碱性的三氟甲磺酸铋(Bi(OTf)_(3))水系电解质.得益于三电子反应和相对于标准氢电极+0.32 V的高电位,铋金属负极具有383 mA h g^(−1)的高比容量和1000次循环的良好稳定性,以及99.6%高库仑效率.铋金属负极在Bi(OTf)_(3)电解液中无腐蚀、钝化和析氢等副反应.此外,非碱性的铋-空气电池通过三氧化二铋(Bi_(2)O_(3))的可逆形成/分解,在环境空气中实现了长期运行稳定性(>200 h).这项工作为探索新型水系金属空气电池作为安全稳定的电源系统提供了新思路.展开更多
Artificial synapse devices with co-location memory and logic functions have attracted enormous attention since they are the indispensable components for neuromorphic computing systems[1].Extensive efforts have been ma...Artificial synapse devices with co-location memory and logic functions have attracted enormous attention since they are the indispensable components for neuromorphic computing systems[1].Extensive efforts have been made to mimic neural electric pulse patterns through solid-state devices like two-terminal memristors and three-terminal transistors.展开更多
Platinum-modified carbon nanotube(CNT) fibers with controlled platinum weight percentages were synthesized via an electrochemical deposition method. Platinum nanoparticles can be uniformly deposited on the surface of ...Platinum-modified carbon nanotube(CNT) fibers with controlled platinum weight percentages were synthesized via an electrochemical deposition method. Platinum nanoparticles can be uniformly deposited on the surface of the aligned CNTs in the fiber, which possesses an efficient improved catalytic activity in the reduction of I3-/I- compared with other fiber materials such as a carbon fiber without the aligned nanostructure. The hybrid CNT fiber was further used as a counter electrode to fabricate fiber-shaped dye-sensitized solar cell(DSSC). A maximal power conversion efficiency of 8.10% was achieved, compared with that of 4.91% for a bare aligned CNT fiber and 5.50% for a platinum-modified carbon fiber as the counter electrode under the same condition.展开更多
基金financially supported by the National Natural Science Foundation of China (52103300)Guangdong Basic and Applied Basic Research Foundation (2023A1515010572)Shenzhen Science and Technology Program (JCYJ20210324132806017 and GXWD20220811163904001)。
基金supported by the Ministry of Science and Technology of the People's Republic of China(MOST)(2022YFA1203001,2022YFA1203002)National Natural Science Foundation of China(NSFC)(T2321003,22335003,T2222005,22175042)Science and Technology Commission of Shanghai Municipality(STCSM)(21511104900)。
文摘Smart electronic textiles with electronic functions like displaying can provide transformative opportunities for wearable devices that traditional rigid devices are hard to realize.A general strategy of enabling textiles to display is weaving light-emitting fibers into textiles and designing control circuits.However,it remains challenging for the current electronic textiles to display full-color images and videos.Here,we demonstrate a large-area integrated electronic textile system(with a size of 72 cm×50 cm)by weaving light-emitting diode(LED)fibers,touch-sensing fibers and polyester fibers,which could display full-color images(with a gamut of 117.6%NTSC)and continuous videos(with a refresh rate of 11.7 Hz)by designing low-voltage supply mode and parallelly transmitting circuits.After integration of touch-sensing fibers,such textile system could achieve various touch display and interactive functions like smart phones or computers,including hand input of text,hand painting,computing and playing games.The stability and durability of textile system withstanding 5000 bending cycles was also demonstrated for wearable applications.The integrated electronic textile system shows similar flexibility and breathability with regular textiles,which is promising to serve as new human-machine interface to change the way in which people interact with electronics.
基金supported by the Minstry of Science and Technology(2022YFA1203001,2022YFA1203002 and 2023YFC2410900)the National Natural Science Foundation of China(T2321003,22335003,T2222005 and 22175042)Science&Technology Commission of Shanghai Municipality(21511104900,20JC1414902 and 23490713500).
基金financially supported by the Science and Technology Commission of Shanghai Municipality(STCSM,21511104900 and 20JC1414902)the National Natural Science Foundation of China(52222310).
文摘水系金属空气电池具有理论能量密度高、安全性高等优点,但受限于金属阳极(如锌、铁、铝、镁)的电化学不可逆性以及碱性电解质对大气中二氧化碳的化学不稳定性.本工作首次设计了一种可充电的铋-空气电池,该电池使用了非碱性的三氟甲磺酸铋(Bi(OTf)_(3))水系电解质.得益于三电子反应和相对于标准氢电极+0.32 V的高电位,铋金属负极具有383 mA h g^(−1)的高比容量和1000次循环的良好稳定性,以及99.6%高库仑效率.铋金属负极在Bi(OTf)_(3)电解液中无腐蚀、钝化和析氢等副反应.此外,非碱性的铋-空气电池通过三氧化二铋(Bi_(2)O_(3))的可逆形成/分解,在环境空气中实现了长期运行稳定性(>200 h).这项工作为探索新型水系金属空气电池作为安全稳定的电源系统提供了新思路.
文摘Artificial synapse devices with co-location memory and logic functions have attracted enormous attention since they are the indispensable components for neuromorphic computing systems[1].Extensive efforts have been made to mimic neural electric pulse patterns through solid-state devices like two-terminal memristors and three-terminal transistors.
基金supported by the Ministry of Science and Technology of China (2011CB932503)the National Natural Science Foundation of China (21225417)+3 种基金STCSM (12nm0503200)Fok Ying Tong Education Foundationthe Program for Special Appointments of Professors at Shanghai Institutions of Higher Learningthe Program for Outstanding Young Scholars from the Organization Department of the CPC Central Committee
文摘Platinum-modified carbon nanotube(CNT) fibers with controlled platinum weight percentages were synthesized via an electrochemical deposition method. Platinum nanoparticles can be uniformly deposited on the surface of the aligned CNTs in the fiber, which possesses an efficient improved catalytic activity in the reduction of I3-/I- compared with other fiber materials such as a carbon fiber without the aligned nanostructure. The hybrid CNT fiber was further used as a counter electrode to fabricate fiber-shaped dye-sensitized solar cell(DSSC). A maximal power conversion efficiency of 8.10% was achieved, compared with that of 4.91% for a bare aligned CNT fiber and 5.50% for a platinum-modified carbon fiber as the counter electrode under the same condition.
