We systematically investigate the polarization gradient cooling （PGC） process in an optical molasses of ultracold cesium atoms. The SR mode for changing the cooling laser, which means that the cooling laser frequenc...We systematically investigate the polarization gradient cooling （PGC） process in an optical molasses of ultracold cesium atoms. The SR mode for changing the cooling laser, which means that the cooling laser frequency is stepped to the setting value while its intensity is ramped, is found to be the best for the PGC, compared with other modes studied. We verify that the heating effect of the cold atoms, which appears when the cooling laser intensity is lower than the saturation intensity, arises from insufficient polarization gradient cooling. Finally, an exponential decay function with a statistical explanation is introduced to explain the dependence of the cold atom temperature on the PGC interaction time.展开更多
We report on the observation of ultracold ground electric-state cesium molecules produced directly in a magneto-optical trap with a good signal-to-noise ratio. These molecules arise from the photoassociation of magnet...We report on the observation of ultracold ground electric-state cesium molecules produced directly in a magneto-optical trap with a good signal-to-noise ratio. These molecules arise from the photoassociation of magneto-optical trap lasers and they are detected by resonantly enhanced multiphoton ionization technology. The production rate of ultracold cesium molecules is up to 4× 10^4 s-1. We measure the characteristic time of the ground electric-state cesium molecules generated in the experiment and investigate the Cs2＋ molecular ion intensity as a function of the trapping laser intensity and the ionization pulse laser energy. We conclude that the production of cold cesium molecules may be enhanced by using appropriate experimental parameters, which is useful for future experiments involving the production and trapping of ultracold ground electric-state molecules.展开更多
We present a simple, robust, space-adjustable dark magneto-optical trap(MOT) for the efficient production of heteronuclear molecules. Double-mixed beams made up of repumping beams and depumping beams propagate in near...We present a simple, robust, space-adjustable dark magneto-optical trap(MOT) for the efficient production of heteronuclear molecules. Double-mixed beams made up of repumping beams and depumping beams propagate in nearly opposite directions in the dark MOT. This optical arrangement can easily adjust the spatial positions of two clouds by changing the power ratio of the two repumping beams, and ensure a good overlap, which is very necessary for the production of heteronuclear molecules. The imaging of cold atoms by camera and the collisioninduced loss rate obtained by recording the loading curve of the cold atoms show that we obtain a perfect overlap of atom clouds. The number of Rb Cs molecules with the double-mixed beams is improved by 70%, which is higher than the one with the single-mixed beam.展开更多
Rydberg atoms have been widely investigated due to their large size,long radiative lifetime,huge polarizability and strong dipole-dipole interactions.The position information of Rydberg atoms provides more possibiliti...Rydberg atoms have been widely investigated due to their large size,long radiative lifetime,huge polarizability and strong dipole-dipole interactions.The position information of Rydberg atoms provides more possibilities for quantum optics research,which can be obtained under the localization method.We study the behavior of three-dimensional(3D)Rydberg atom localization in a four-level configuration with the measurement of the spatial optical absorption.The atomic localization precision depends strongly on the detuning and Rabi frequency of the involved laser fields.A 100%probability of finding the Rydberg atom at a specific 3D position is achieved with precision of~0.031λ.This work demonstrates the possibility for achieving the 3D atom localization of the Rydberg atom in the experiment.展开更多
We experimentally observe the high resolution direct frequency comb spectroscopy using counter-propagating broadband femtosecond pulses on two-photon transitions in room-temperature ^87 Rb atoms. The Doppler broad- en...We experimentally observe the high resolution direct frequency comb spectroscopy using counter-propagating broadband femtosecond pulses on two-photon transitions in room-temperature ^87 Rb atoms. The Doppler broad- ened background is effectively eliminated with the pulse shaping method and the spectrum modulation technique. The combination of the pulse shaping method and the spectra modulation technique provides a potential approachto reduce background of at least 99%.展开更多
In this paper, ultracold atoms and molecules in a dark magneto-optical trap （MOT） are studied via depumping the cesium cold atoms into the dark hyperfine ground state. The collision rate is reduced to 0.45 s-1 and t...In this paper, ultracold atoms and molecules in a dark magneto-optical trap （MOT） are studied via depumping the cesium cold atoms into the dark hyperfine ground state. The collision rate is reduced to 0.45 s-1 and the density of the atoms is increased to 5.6 × 1011 cm-3 when the fractional population of the atoms in the bright hyperfine ground state is as low as 0.15. The vibrational spectra of the ultracold cesium molecules are also studied in a standard MOT and in a dark MOT separately. The experimental results are analyzed by using the perturbative quantum approach.展开更多
We demonstrate the generation of the coherent 420 nm laser via parametric four-wave mixing process in Rb vapor.A single 778 nm laser with circular polarization is directly injected into a high-density atomic vapor,whi...We demonstrate the generation of the coherent 420 nm laser via parametric four-wave mixing process in Rb vapor.A single 778 nm laser with circular polarization is directly injected into a high-density atomic vapor,which drives the atoms from the 5S1/2 state to the 5D5/2 state with monochromatic two-photon transition.The frequency up-conversion laser is generated by the parametric four-wave mixing process under the phase matching condition.This coherent laser is firstly certified by the knife-edge method and a narrow range grating spectrometer.Then the generated laser power is investigated in terms of the power and frequency of the incoming beam as well as the density of the atoms.Finally,a 420 nm coherent laser with power of 19μW and beam quality of Mx^2=1.32,My^2=1.37 is obtained with optimal experimental parameters.This novel laser shows potential prospects in the measurement of material properties,information storage,and underwater optical communication.展开更多
We investigate the production of ultracold ground state x^1∑7＋（u = 0） RbCs molecules in the lowest vibrational level via short-range photoassociation followed by spontaneous emission. The starting point is the las...We investigate the production of ultracold ground state x^1∑7＋（u = 0） RbCs molecules in the lowest vibrational level via short-range photoassociation followed by spontaneous emission. The starting point is the laser cooled 85Rb and laa cs atoms in a dual species, forced dark magneto-optical trap. The special intermediate level （5）O＋ （u = 10） correlated to the （2）311 electric state is achieved by the photoassociation process. The formed ground state X1∑＋ （u = 0） molecule is resonantly excited to the 2111 intermediate state by a 651 nm pulse laser and is ionized by a 532nm pulse laser and then detected by the time-of-flight mass spectrum. Saturation of the photoionization spectroscopy at large ionization laser energy is observed and the ionization efficiency is obtained from the fitting. The production of ultracold ground state 85Rblaacs molecules is facilitative for the further research about the manipulation of ultracold molecules in the rovibrational ground state.展开更多
We present a method to precisely determine the hyperfine structure constants of the rubidium 5D（5/2） and 7S（1/2） states in a cascade atomic system. The probe laser is coupled to the 5S（1/2）→ 5P（3/2） hyperfine...We present a method to precisely determine the hyperfine structure constants of the rubidium 5D（5/2） and 7S（1/2） states in a cascade atomic system. The probe laser is coupled to the 5S（1/2）→ 5P（3/2） hyperfine transition, while the coupling laser is scanned over the 5P（3/2）→ 5D（5/2）（7S（1/2）） transition. The high-resolution double-resonance optical pumping spectra are obtained with two counter-propagating laser beams acting on rubidium vapor. The hyperfine splitting structures are accurately measured by an optical frequency ruler based on the acousto-optic modulator, thus, the magnetic dipole hyperfine coupling constant A and quadrupole coupling constant B are determined. It is of great significance for the atomic hyperfine structure and fundamental physics research.展开更多
Ultracold polar RbCs molecules are produced via photoassociation in a laser-cooled mixture of ^85Rb and ^133Cs atoms. The a3∑＋ state molecules which decay from electronically excited （2）0- state RbCs molecules are...Ultracold polar RbCs molecules are produced via photoassociation in a laser-cooled mixture of ^85Rb and ^133Cs atoms. The a3∑＋ state molecules which decay from electronically excited （2）0- state RbCs molecules are detected by resonance- enhanced two-photon ionization. The new rovibrational levels （v = 189, 190） in the （2）0- state are also observed, which exist in theory and have not been observed in experiments yet. The corresponding rotational constants are measured by photoassociation spectroscopy, which are consistent with theoretical calculations using a nonrigid rotor model.展开更多
Double resonance optical pumping spectroscopy has an outstanding advantage of high signal-to-noise ratio, thus having potential applications in precision measurement. With the counter propagated 780nm and 776nm laser ...Double resonance optical pumping spectroscopy has an outstanding advantage of high signal-to-noise ratio, thus having potential applications in precision measurement. With the counter propagated 780nm and 776nm laser beams acting on a rubidium vapor cell, the high resolution spectrum of 5S1/2 - 5P3/2 - 5D5/2 ladder-type transition of ST Rb atoms is obtained by monitoring the population of the 5S1/2 ground state. The dependence of the spectroscopy lineshape on the probe and coupling fields are comprehensively studied in theory and experiment. This research is helpful for measurement of fundamental physical constants by high resolution spectroscopy.展开更多
We have produced ultracold polar RbCs molecules via photoassociation starting from laser-cooled 85Rb and 133Cs atoms in a dual−species,forced dark magneto-optical trap.The formed electronically excited RbCs∗molecules ...We have produced ultracold polar RbCs molecules via photoassociation starting from laser-cooled 85Rb and 133Cs atoms in a dual−species,forced dark magneto-optical trap.The formed electronically excited RbCs∗molecules correlated to the Rb(5S_(1/2))+Cs(6P_(1/2))dissociation limit are observed by trap loss spectroscopy.Following the decay of these excited RbCs*molecules,the formed ground state molecules are directly ionized by a two-photon single-color pulse dye laser,which is a new ionization mechanism for ground state RbCs molecules and thence detected by time-of-flight mass spectroscopy.展开更多
基金supported by the National Basic Research Program of China(Grant Nos.2012CB921603 and 2010CB923103)the International Science &Technology Cooperation Program of China(Grant No.2011DFA12490)+2 种基金the National Natural Science Foundation of China(Grant Nos.11304189,61378015,and 61275209)the Project for Excellent Research Team of the National Natural Science Foundation of China(Grant No.61121064)the Program for Changjiang Scholars,China,and the Innovative Research Team in University,China(Grant No.IRT13076)
文摘We systematically investigate the polarization gradient cooling （PGC） process in an optical molasses of ultracold cesium atoms. The SR mode for changing the cooling laser, which means that the cooling laser frequency is stepped to the setting value while its intensity is ramped, is found to be the best for the PGC, compared with other modes studied. We verify that the heating effect of the cold atoms, which appears when the cooling laser intensity is lower than the saturation intensity, arises from insufficient polarization gradient cooling. Finally, an exponential decay function with a statistical explanation is introduced to explain the dependence of the cold atom temperature on the PGC interaction time.
基金supported by the National Key Fundamental Basic Research Program of China (Grant No. 2006CB921603)the Major Program of National Natural Science Foundation of China (Grant No. 10934004)+3 种基金the National Natural Science Foundation of China (Grant Nos. 60978018,60808009,61008012,and 60978001)the New Teacher Fund of the Ministry of Education of China(Grant No. 200801081021)the National Natural Science Foundation of China for Excellent Research Team (Grant No. 60821004)the Natural Science Foundation of Shanxi Province of China (Grant No. 2009011059-2)
文摘We report on the observation of ultracold ground electric-state cesium molecules produced directly in a magneto-optical trap with a good signal-to-noise ratio. These molecules arise from the photoassociation of magneto-optical trap lasers and they are detected by resonantly enhanced multiphoton ionization technology. The production rate of ultracold cesium molecules is up to 4× 10^4 s-1. We measure the characteristic time of the ground electric-state cesium molecules generated in the experiment and investigate the Cs2＋ molecular ion intensity as a function of the trapping laser intensity and the ionization pulse laser energy. We conclude that the production of cold cesium molecules may be enhanced by using appropriate experimental parameters, which is useful for future experiments involving the production and trapping of ultracold ground electric-state molecules.
基金supported by the National 973 Program of China(No.2012CB921603)the National Natural Science Foundation of China(Nos.61275209,11304189,61378015,and 11434007)+1 种基金the NSFC Project for Excellent Research Team(No.61121064)PCSIRT(No.IRT13076)
文摘We present a simple, robust, space-adjustable dark magneto-optical trap(MOT) for the efficient production of heteronuclear molecules. Double-mixed beams made up of repumping beams and depumping beams propagate in nearly opposite directions in the dark MOT. This optical arrangement can easily adjust the spatial positions of two clouds by changing the power ratio of the two repumping beams, and ensure a good overlap, which is very necessary for the production of heteronuclear molecules. The imaging of cold atoms by camera and the collisioninduced loss rate obtained by recording the loading curve of the cold atoms show that we obtain a perfect overlap of atom clouds. The number of Rb Cs molecules with the double-mixed beams is improved by 70%, which is higher than the one with the single-mixed beam.
基金the National R&D Program of China(Grant No.2017YFA0304203)the National Natural Science Foundation of China(Grant Nos.61875112,61705122,62075121,and 91736209)+1 种基金the Program for Sanjin Scholars of Shanxi Province,the Key Research and Development Program of Shanxi Province for International Cooperation(Grant No.201803D421034)Shanxi Scholarship Council of China(Grant Nos.2020-073),and 1331KSC.
文摘Rydberg atoms have been widely investigated due to their large size,long radiative lifetime,huge polarizability and strong dipole-dipole interactions.The position information of Rydberg atoms provides more possibilities for quantum optics research,which can be obtained under the localization method.We study the behavior of three-dimensional(3D)Rydberg atom localization in a four-level configuration with the measurement of the spatial optical absorption.The atomic localization precision depends strongly on the detuning and Rabi frequency of the involved laser fields.A 100%probability of finding the Rydberg atom at a specific 3D position is achieved with precision of~0.031λ.This work demonstrates the possibility for achieving the 3D atom localization of the Rydberg atom in the experiment.
基金Supported by the National Basic Research Program of China under Grant No 2012CB921603the Program for Changjiang Scholars and Innovative Research Team in University of Ministry of Education of China under Grant No IRT13076the National Natural Science Foundation of China under Grant Nos 61378049,10934004,11404198,61575116 and 61505100
文摘We experimentally observe the high resolution direct frequency comb spectroscopy using counter-propagating broadband femtosecond pulses on two-photon transitions in room-temperature ^87 Rb atoms. The Doppler broad- ened background is effectively eliminated with the pulse shaping method and the spectrum modulation technique. The combination of the pulse shaping method and the spectra modulation technique provides a potential approachto reduce background of at least 99%.
基金Project supported by the National Basic Research Program of China (Grant No. 2012CB921603)the International Science & Technology Cooperation Program of China (Grant No. 2011DFA12490)+1 种基金the National Natural Science Foundation of China (Grant Nos.10934004,60978001,60978018,60808009,61078001,and 61008012)the Natural Science Foundation of Shanxi Province,China (Grant No. 2011011004)
文摘In this paper, ultracold atoms and molecules in a dark magneto-optical trap （MOT） are studied via depumping the cesium cold atoms into the dark hyperfine ground state. The collision rate is reduced to 0.45 s-1 and the density of the atoms is increased to 5.6 × 1011 cm-3 when the fractional population of the atoms in the bright hyperfine ground state is as low as 0.15. The vibrational spectra of the ultracold cesium molecules are also studied in a standard MOT and in a dark MOT separately. The experimental results are analyzed by using the perturbative quantum approach.
基金Project supported by the National R&D Program of China(Grant No.2017YFA0304203)the National Natural Science Foundation of China(Grant Nos.61875112,61705122,91736209,and 61728502)+2 种基金the Program for Sanjin Scholars of Shanxi Province,China,the Applied Basic Research Project of Shanxi Province,China(Grant No.201701D221004)the Key Research and Development Program of Shanxi Province for International Cooperation,China(Grant No.201803D421034)1331KSC。
文摘We demonstrate the generation of the coherent 420 nm laser via parametric four-wave mixing process in Rb vapor.A single 778 nm laser with circular polarization is directly injected into a high-density atomic vapor,which drives the atoms from the 5S1/2 state to the 5D5/2 state with monochromatic two-photon transition.The frequency up-conversion laser is generated by the parametric four-wave mixing process under the phase matching condition.This coherent laser is firstly certified by the knife-edge method and a narrow range grating spectrometer.Then the generated laser power is investigated in terms of the power and frequency of the incoming beam as well as the density of the atoms.Finally,a 420 nm coherent laser with power of 19μW and beam quality of Mx^2=1.32,My^2=1.37 is obtained with optimal experimental parameters.This novel laser shows potential prospects in the measurement of material properties,information storage,and underwater optical communication.
基金Supported by the National Basic Research Program of China under Grant No 2012CB921603the National Natural Science Foundation of China under Grant Nos 61275209,11304189,61378015 and 11434007+1 种基金the National Natural Science Foundation for Excellent Research Team under Grant No 61121064the Program for Changjiang Scholars and Innovative Research Team in University under Grant No IRT13076
文摘We investigate the production of ultracold ground state x^1∑7＋（u = 0） RbCs molecules in the lowest vibrational level via short-range photoassociation followed by spontaneous emission. The starting point is the laser cooled 85Rb and laa cs atoms in a dual species, forced dark magneto-optical trap. The special intermediate level （5）O＋ （u = 10） correlated to the （2）311 electric state is achieved by the photoassociation process. The formed ground state X1∑＋ （u = 0） molecule is resonantly excited to the 2111 intermediate state by a 651 nm pulse laser and is ionized by a 532nm pulse laser and then detected by the time-of-flight mass spectrum. Saturation of the photoionization spectroscopy at large ionization laser energy is observed and the ionization efficiency is obtained from the fitting. The production of ultracold ground state 85Rblaacs molecules is facilitative for the further research about the manipulation of ultracold molecules in the rovibrational ground state.
基金supported by the National Key R&D Program of China(No.2017YFA0304203)the National Natural Science Foundation of China(Nos.61575116,61705122,61728502,91736209,and 11434007)+3 种基金the Changjiang Scholars and Innovative Research Team in University of Ministry of Education of China(No.IRT13076)the Program for Sanjin Scholars of Shanxi Provincethe Applied Basic Research Project of Shanxi Province(No.201701D221004)the Fund for Shanxi‘1331 Project’Key Subjects Construction
文摘We present a method to precisely determine the hyperfine structure constants of the rubidium 5D（5/2） and 7S（1/2） states in a cascade atomic system. The probe laser is coupled to the 5S（1/2）→ 5P（3/2） hyperfine transition, while the coupling laser is scanned over the 5P（3/2）→ 5D（5/2）（7S（1/2）） transition. The high-resolution double-resonance optical pumping spectra are obtained with two counter-propagating laser beams acting on rubidium vapor. The hyperfine splitting structures are accurately measured by an optical frequency ruler based on the acousto-optic modulator, thus, the magnetic dipole hyperfine coupling constant A and quadrupole coupling constant B are determined. It is of great significance for the atomic hyperfine structure and fundamental physics research.
基金supported by the National Basic Research Program of China (Grant No. 2012CB921603)the International Science & Technology Cooperation Program of China (Grant No. 2011DFA12490)+1 种基金the National Natural Science Foundation of China (Grant Nos. 61275209, 10934004, and 11004125)the National Natural Science Foundation for Excellent Research Team, China (Grant No. 61121064)
文摘Ultracold polar RbCs molecules are produced via photoassociation in a laser-cooled mixture of ^85Rb and ^133Cs atoms. The a3∑＋ state molecules which decay from electronically excited （2）0- state RbCs molecules are detected by resonance- enhanced two-photon ionization. The new rovibrational levels （v = 189, 190） in the （2）0- state are also observed, which exist in theory and have not been observed in experiments yet. The corresponding rotational constants are measured by photoassociation spectroscopy, which are consistent with theoretical calculations using a nonrigid rotor model.
基金Supported by the National Key R&D Program of China under Grant No 2017YFA0304203the National Natural Science Foundation of China under Grant Nos 61575116,61705122,61728502,91736209 and 11434007+2 种基金the Changjiang Scholars and Innovative Research Team in University of Ministry of Education of China under Grant No IRT13076the Program for Sanjin Scholars of Shanxi Province,the Applied Basic Research Project of Shanxi Province under Grant No 201701D221004the Fund for Shanxi ‘1331 Project’ Key Subjects Construction
文摘Double resonance optical pumping spectroscopy has an outstanding advantage of high signal-to-noise ratio, thus having potential applications in precision measurement. With the counter propagated 780nm and 776nm laser beams acting on a rubidium vapor cell, the high resolution spectrum of 5S1/2 - 5P3/2 - 5D5/2 ladder-type transition of ST Rb atoms is obtained by monitoring the population of the 5S1/2 ground state. The dependence of the spectroscopy lineshape on the probe and coupling fields are comprehensively studied in theory and experiment. This research is helpful for measurement of fundamental physical constants by high resolution spectroscopy.
基金by the National Key Fundamental Basic Research Program of China(2006CB921603)Major Program of the National Natural Science Foundation of China(10934004)+2 种基金the National Natural Science Foundation of China(60978018,60808009,61008012,and 60978001)the New Teacher Fund of Ministry of Education of China(200801081021)NSFC Project for Excellent Research Team(Grant No 60821004).
文摘We have produced ultracold polar RbCs molecules via photoassociation starting from laser-cooled 85Rb and 133Cs atoms in a dual−species,forced dark magneto-optical trap.The formed electronically excited RbCs∗molecules correlated to the Rb(5S_(1/2))+Cs(6P_(1/2))dissociation limit are observed by trap loss spectroscopy.Following the decay of these excited RbCs*molecules,the formed ground state molecules are directly ionized by a two-photon single-color pulse dye laser,which is a new ionization mechanism for ground state RbCs molecules and thence detected by time-of-flight mass spectroscopy.
