Based on hourly precipitation data in eastern China in the warm season during 1961-2000,spatial distributions of frequency for 20 mm h 1 and 50 mm h 1 precipitation were analyzed,and the criteria of short-duration rai...Based on hourly precipitation data in eastern China in the warm season during 1961-2000,spatial distributions of frequency for 20 mm h 1 and 50 mm h 1 precipitation were analyzed,and the criteria of short-duration rainfall events and severe rainfall events are discussed.Furthermore,the percentile method was used to define local hourly extreme precipitation;based on this,diurnal variations and trends in extreme precipitation were further studied.The results of this study show that,over Yunnan,South China,North China,and Northeast China,the most frequent extreme precipitation events occur most frequently in late afternoon and/or early evening.In the Guizhou Plateau and the Sichuan Basin,the maximum frequency of extreme precipitation events occurs in the late night and/or early morning.And in the western Sichuan Plateau,the maximum frequency occurs in the middle of the night.The frequency of extreme precipitation （based on hourly rainfall measurements） has increased in most parts of eastern China,especially in Northeast China and the middle and lower reaches of the Yangtze River,but precipitation has decreased significantly in North China in the past 50 years.In addition,stations in the Guizhou Plateau and the middle and lower reaches of the Yangtze River exhibit significant increasing trends in hourly precipitation extremes during the nighttime more than during the daytime.展开更多
Chengdu is a megacity in the southwest of China with high ozone(O_3) mixing ratio.Observation of volatile organic compounds(VOCs), NO_2 and O_3 with high temporal resolution was conducted in Chengdu to investigate the...Chengdu is a megacity in the southwest of China with high ozone(O_3) mixing ratio.Observation of volatile organic compounds(VOCs), NO_2 and O_3 with high temporal resolution was conducted in Chengdu to investigate the chemical processes and causes of high O_3 levels. The hourly mixing ratios of VOCs, NO2, and O_3 were monitored by an online system from 28 August to 7 October, 2016. According to meteorological conditions,Chengdu, with relative warm weather and low wind speed, is favorable to O_3 formation.Part of the O_3 in Chengdu may be transported from the downtown area. In O_3 episodes,the average mixing ratios of NO_2 and O_3 were 20.20 ppbv and 47.95 ppbv, respectively. In non-O_3 episodes, the average mixing ratios of NO_2 and O_3 were 16.38 ppbv and 35.15 ppbv,respectively. The average mixing ratio of total VOCs(TVOCs) was 40.29 ppbv in non-O_3 episodes, which was lower than that in O_3 episodes(53.19 ppbv). Alkenes comprised51.7% of the total O_3 formation potential(OFP) in Chengdu, followed by aromatics which accounted for 24.2%. Ethylene, trans-pentene, propene, and BTEX(benzene, ethylbenzene,toluene, m/p-xylene, o-xylene) were also major contributors to the OFP in Chengdu. In O_3 episodes, intensive secondary formations were observed during the campaign. Oxygenated VOCs(OVOCs), such as acetone, Methylethylketone(MEK), and Methylvinylketone(MVK)were abundant. Isoprene rapidly converted to MVK and Methacrolein(MACR) during O_3 episodes. Acetone was mainly the oxidant of C3-C5 hydrocarbons.展开更多
The present study examined the diurnal variations of summer precipitation in the Beijing area by usingsubdaily precipitation and wind observations. A combined effect of topography and urbanization on thecharacteristic...The present study examined the diurnal variations of summer precipitation in the Beijing area by usingsubdaily precipitation and wind observations. A combined effect of topography and urbanization on thecharacteristics of diurnal variations was suggested. It was shown that stations located in the plain areaexhibited typical night rain peaks, whereas those in the mountainous area exhibited clear afternoon peaks ofprecipitation diurnal variations. The precipitation peaks were associated with wind fields around the Beijingarea, which were found to be highly modulated by mountain-valley circulation and urban-country circulation.The lower-tropospheric wind exhibited a clear diurnal shift in its direction from north at 0800 LST to southat 2000 LST, which reflected mountain-valley circulation. The transitions from valley to mountain windand the opposite generally happened after sunset and sunrise, respectively, and both occurred earlier for thestations located closer to mountains. By comparing the diurnal variations of precipitation at stations in anortheast suburb, an urban area, and a southwest suburb, it was revealed that the northeast suburb grouphad the highest normalized rainfall frequency, but the southwest group had the lowest from late afternoon tolate evening. On the contrary, in the early morning from about 0200 to 1000 LST, the southwest group andurban group had the highest normalized rainfall frequency. This pattern might originate from the combinedeffects of mountain-valley topography and urbanization.展开更多
Short-duration heavy rainfall（SDHR） is a type of severe convective weather that often leads to substantial losses of property and life. We derive the spatiotemporal distribution and diurnal variation of SDHR over Ch...Short-duration heavy rainfall（SDHR） is a type of severe convective weather that often leads to substantial losses of property and life. We derive the spatiotemporal distribution and diurnal variation of SDHR over China during the warm season（April–September） from quality-controlled hourly raingauge data taken at 876 stations for 19 yr（1991–2009）, in comparison with the diurnal features of the mesoscale convective systems（MCSs） derived from satellite data. The results are as follows. 1） Spatial distributions of the frequency of SDHR events with hourly rainfall greater than 10–40 mm are very similar to the distribution of heavy rainfall（daily rainfall 50 mm） over China's Mainland. 2） SDHR occurs most frequently in South China such as southern Yunnan, Guizhou, and Jiangxi provinces, the Sichuan basin, and the lower reaches of the Yangtze River, among others. Some SDHR events with hourly rainfall 50 mm also occur in northern China, e.g., the western Xinjiang and central-eastern Inner Mongolia. The heaviest hourly rainfall is observed over the Hainan Island with the amount reaching over 180 mm. 3） The frequency of the SDHR events is the highest in July, followed by August. Analysis of pentad variations in SDHR reveals that SDHR events are intermittent, with the fourth pentad of July the most active. The frequency of SDHR over China's Mainland increases slowly with the advent of the East Asian summer monsoon, but decreases rapidly with its withdrawal. 4） The diurnal peak of the SDHR activity occurs in the later afternoon（1600–1700 Beijing Time（BT））, and the secondary peak occurs after midnight（0100–0200 BT） and in the early morning（0700–0800 BT）; whereas the diurnal minimum occurs around late morning till noon（1000–1300 BT）. 5） The diurnal variation of SDHR exhibits generally consistent features with that of the MCSs in China, but the active periods and propagation of SDHR and MCSs difer in diferent regions. The number and duration of local maxima in the d展开更多
An intensive observation of organic carbon （OC） and element carbon （EC） in PM10 and gaseous materials （SO2, CO, and O3,） was conducted continuously to assess the characteristics of wintertime carbonaceous aeroso...An intensive observation of organic carbon （OC） and element carbon （EC） in PM10 and gaseous materials （SO2, CO, and O3,） was conducted continuously to assess the characteristics of wintertime carbonaceous aerosols in an urban area of Beijing, China. Results showed that the averaged total carbon （TC） and PM10 concentrations in observation period are 30.2±120.4 and 172.6±198.3 μ/m^3 respectively. Average OC concentration in nighttime （24.9±19.6 μ/m^3 was 40% higher than that in daytime （17.7±10.9 μ/m^3. Average EC concentrations in daytime （8.8±15.2 μ/m^3 was close to that in nighttime （8.9±15.1 μ/m^3. The OC/EC ratios in nighttime ranging from 2.4 to 2.7 are higher than that in daytime ranging from 1.9 to 2.0. The concentrations of OC, EC, PM10 were low with strong winds and high with weak winds. The OC and EC were well correlated with PM10, CO and SO2, which implies they have similar sources. OC and EC were not well correlated with O3. By considering variation of OC/EC ratios in daytime and night time, correlations between OC and O3, and meteorological condition, we speculated that OC and EC in Beijing PM10 were emitted as the primary particulate form. Emission of motor vehicle with low OC/EC ratio and coal combustion sources with high OC/EC ratio are probably the dominant sources for carbonaceous aerosols in Beijing in winter. A simple method was used to estimate the relative contribution of sources to carbonaceous aerosols in Beijing PM10. Motor vehicle source accounts for 80% and 68%, while coal combustion accounts for 20% and 32% in daytime and nighttime, respectively in Beijing. Averagely, the motor vehicle and coal combustion accounted for 74% and 26%, respectively, for carbonaceous aerosols during the observation period. It points to the motor vehicle is dominant emission for carbonaceous aerosols in Beijing PM10 in winter period, which should be paid attention to control high level of PM10 in Beijing effectively.展开更多
The aerosol number concentration and size distribution were measured with the newly developed Wide-range Particle Spectrometer in summer and winter of 2006 at the urban site of Jinan City. Here reported the characteri...The aerosol number concentration and size distribution were measured with the newly developed Wide-range Particle Spectrometer in summer and winter of 2006 at the urban site of Jinan City. Here reported the characteristics of fine particles of the different observation seasons. Relative high number concentrations for the particles in the diameter range of 10-500 nm were observed in both seasons. It was found that the dominant number distributed in particle diameter smaller than 100 nm and the percentage over the number concentration of all air particles is much higher than what has been measured in other urban sites over the world. The number mean diameter in summer was much smaller than in winter, strongly suggesting the different origin of ultrafine particles in different seasons. That is, particles in ultrafine mode mainly came from nucleation and new particle formation in summer while from traffic emission in winter. The diurnal variation also supported this point. Number concentration in the diameter range of 10-200 um got their peak values at noontime, well correlated with the mixing ratio of SO2 and the intensity of solar radiation in summer. While in winter, those in the same diameter range showed the main peaks during the traffic hours happened in the morning and evening.展开更多
Diurnal variations of two mountain-plain solenoid （MPS） circulations associated with ＂first-step＂ terrain [Tibetan Plateau （TP）] and ＂second-step＂ terrain （high mountains between the TP and ＂east plains＂） ...Diurnal variations of two mountain-plain solenoid （MPS） circulations associated with ＂first-step＂ terrain [Tibetan Plateau （TP）] and ＂second-step＂ terrain （high mountains between the TP and ＂east plains＂） in China and their influence on the south west vortex （SWV） and the mei-yu front vortex （MYFV） were investigated via a semi-idealized mesoscale numerical model [Weather Research and Forecasting （WRF）] simulation integrated with ten-day average fields （mei-yu period of 1-10 July 2007）. The simulations successfully reproduced two MPS circulations related to first and second-step terrain, diurnal vari- ations from the eastern edge of the TP to the Yangtze River-Huaihe River valleys （YHRV）, and two precipitation maximum centers related to the SWV, MYFV. Analyses of the averaged final seven-day simulation showed the different diurnal peaks of precipitation at different regions： from the aftemoon to early evening at the eastern edge of the TP; in the early evening to the next early morning in the Sichuan Basin （SCB）; and in the late evening to the next early morning over the mei-yu front （MYF）. Analyses of individual two-day cases confirmed that the upward branches of the nightlime MPS circulations enhanced the precipitation over the SWV and the MYFV and revealed that the eastward extension of the SWV and its con vection were conducive to triggering the MYFVs. The eastward propagation of a rainfall streak from the eastern edge of the TP to the eastern coastal region was primarily due to a series of convective activities of several systems from west to east, including the MPS between the TP and SCB, the SWV, the MPS between second-step terrain and tile east plains, and the MYFV.展开更多
Climatological characteristics of diurnal variations in summer precipitation over the Asian monsoon region are comprehensively investigated based on the Tropical Rainfall Measuring Mission(TRMM) satellite data during ...Climatological characteristics of diurnal variations in summer precipitation over the Asian monsoon region are comprehensively investigated based on the Tropical Rainfall Measuring Mission(TRMM) satellite data during 1998-2008.The topographic influence on the diurnal variations and phase propagations of maximum precipitation are identified according to spatiotemporal distributions of the amplitude and peak time of the diurnal precipitation.The amplitude and phase of diurnal precipitation show a distinct geographical pattern.Significant diurnal variations occur over most of continental and coastal areas including the Maritime Continent,with the relative amplitude exceeding 40%,indicating that the precipitation peak is 1.4 times the 24-h mean.Over the landside coasts such as southeastern China and Indochina Peninsula,the relative amplitude is even greater than 100%.Although the diurnal variations of summer precipitation over the continental areas are characterized by an afternoon peak(1500-1800 Local Solar Time(LST)),over the central Indochina Peninsula and central and southern Indian Peninsula the diurnal phase is delayed to after 2100 LST,suggesting the diurnal behaviors over these areas different from the general continental areas.The weak diurnal variations with relative amplitudes less than 40% exist mainly over oceanic areas in the western Pacific and most of Indian Ocean,with the rainfall peak mainly occurring from midnight to early morning(0000-0600 LST),indicating a typical oceanic regime characterized by an early morning peak.However,apparent exceptions occur over the South China Sea(SCS),Bay of Bengal(BOB),and eastern Arabian Sea,with the rainfall peak occurring in daytime(0900-1500 LST).Prominent meridional propagations of the diurnal phase exist in South Asia and East Asia.Along the eastern Indian Peninsula,there is not only the southward phase propagation with the peak occurring around 25°N but also the northward phase propagation with the peak beginning with the southernmost continent,and both reach展开更多
The mountain-plains solenoid(MPS) and boundary-layer inertial oscillation(BLO) are two typical regional forcings at the diurnal time scale. Their relative role in regulating the diurnal variations of summer rainfall o...The mountain-plains solenoid(MPS) and boundary-layer inertial oscillation(BLO) are two typical regional forcings at the diurnal time scale. Their relative role in regulating the diurnal variations of summer rainfall over North China and their change under different monsoon conditions are studied using a 19-yr archive of satellite rainfall and reanalysis data. It is shown that both a strong MPS and BLO can increase nocturnal rainfall in the North China plains but exhibit evident regional differences. The MPS-induced nocturnal rainfall is relatively confined to the plains adjacent to mountains from late night to morning, due to the upward branch of the nighttime MPS. In contrast, the BLO-induced nocturnal rainfall strengthens from early evening and is more extensive in early morning over the open plains further east. The contrasting effect in the evening is related to the convergent(divergent) easterly anomaly in the plains under the BLO(MPS). The BLO also induces the relatively strong enhancement of moisture convergence and high humidity by the southerly anomaly at late night. On strong monsoon days, the nocturnal rainfall amount associated with the MPS and BLO increases considerably in the plains.Both regional forcings become effective in regulating the rainfall diurnal cycle with enhanced moisture convergence under monsoon conditions. Their induced diurnal amplitudes of moisture convergence can be comparable to the daily mean by monsoon flow. The regional forcings thus couple with monsoon flow to strengthen rainfall in the plains, particularly from late night to morning. The results highlight that a combination of regional and large-scale forcings can strongly regulate the warm-season climate.展开更多
Based on in-situ time series data from the acoustic Doppler current profiler （ADCP） and thermistor chain in Wenchang area, a sequence of internal solitary wave （ISW） packets was observed in September 2005, propaga...Based on in-situ time series data from the acoustic Doppler current profiler （ADCP） and thermistor chain in Wenchang area, a sequence of internal solitary wave （ISW） packets was observed in September 2005, propagating northwest on the continental shelf of the northwestern South China Sea （SCS）. Corresponding to different stratification of the water column and tidal condition, both elevation and depression ISWs were observed at the same mooring location with amplitude of 35 m and 25 m respectively in different days. Regular arrival of the remarkable ISW packets at approximately the diurnal tidal period and the dominance of diurnal internal waves in the study area, strongly suggest that the main energy source of the waves is the diurnal tide. Notice that the wave packets were all riding on the troughs and shoulders of the internal tides, they were probably generated locally from the shelf break by the evolution of the internal tides due to nonlinear and dispersive effects.展开更多
In this study, records from a 3-yr intensified observational experiment at eight stations along the hillside of Seqilashan over the southeastern Tibetan Plateau were analyzed and combined with records at 28 routine ob...In this study, records from a 3-yr intensified observational experiment at eight stations along the hillside of Seqilashan over the southeastern Tibetan Plateau were analyzed and combined with records at 28 routine observation stations in the Chinese National Meteorological Station Network to investigate the influences of station location on the different diurnal rainfall variations between station records and Tropical Rainfall Measuring Mission （TRMM） data products. The results indicate that the diurnal variation of warm season rainfall is closely related to location of stations. The prevailing nocturnal rainfall peak in observations at routine stations can be largely attributed to the relatively lower location of the stations, which are mostly situated in valleys. The records at Seqilashan stations on hillsides revealed an evident diurnal afternoon peak of warm season rainfall, similar to that indicated by TRMM data. The different diurnal phases between valley and hillside stations are closely related to the orographically induced regional circulations caused by the complex topography over the Tibetan Plateau. The results of this study indicate that the prevailing nocturnal rainfall associated with the relatively lower location of routine observation stations can partially explain the diurnal rainfall variations between observation station records and TRMM data.展开更多
This study was performed at three eutrophic rivers in Southeast China aiming to determine the magnitude and patterns of dissolved N2O concentrations and fluxes over a seasonal （in 2009） and diurnal （24 h） temporal...This study was performed at three eutrophic rivers in Southeast China aiming to determine the magnitude and patterns of dissolved N2O concentrations and fluxes over a seasonal （in 2009） and diurnal （24 h） temporal scale.The results showed that N2O concentrations varied from 0.28 to 0.38 （mean 0.32±0.04）,0.29 to 0.46 （mean 0.37±0.07）,and 2.07 to 3.47 （mean 2.84±0.63） μg N-N2O L-1 in the Fengle,Hangbu and Nanfei rivers,respectively,in the diurnal study performed during the summer of 2008.The study found that mean N2O concentration and estimated N2O flux （67.89 ± 6.71 μg N-N2O m-2 h-1） measured from the Nanfei River with serious urban wastewater pollution was significantly higher than those from the Fengle and the Hangbu Rivers with agricultural runoff.In addition,the seasonal study during June and December of 2009 also showed that the mean N2O concentration （10.59±14.67 μg N-N2O L-1） and flux （236.87±449.74 μg N-N2O m-2 h-1） observed from the Nanfei River were significantly higher than those from the other two rivers.Our study demonstrated both N2O concentrations and fluxes exhibited seasonal and diurnal fluctuations.Over three consecutive days during the summer of 2008,N2O accumulation rates varied within the range of 3.91-7.21,2.76-15.71,and 3.23-30.03 μg N-N2O m-2 h-1 for the Fengle,Hangbu and Nanfei Rivers,respectively,and exponentially decreased with time.展开更多
To investigate the diurnal variation of summer precipitation in the Qilian Mountains in the northeast Tibetan Plateau, the hourly precipitation amount for this region during the summers of 2008-2014 are analyzed using...To investigate the diurnal variation of summer precipitation in the Qilian Mountains in the northeast Tibetan Plateau, the hourly precipitation amount for this region during the summers of 2008-2014 are analyzed using an hourly merged precipitation product at 0.1°×0.1 ° resolution. The main results are as follows. （1） The spatial distribution and temporal variation of mean hourly precipitation amount and frequency are generally similar and hourly precipitations in the eastern and middle portions are larger and more frequent than that in the western portion. The high value area of precipitation intensity is obviously different from that of precipitation amount and frequency. （2） The spatial distribution of daytime precipitation is generally similar to that of nighttime precipitation, and the daytime precipitation is heavier than the nighttime precipitation. （3） The change rate of precipitation has a maximum at 20：00 Beijing time, and a minimum at 12：00. The hourly precipitation amount significantly correlated with frequency, especially for the middle and eastern portions.展开更多
A field campaign on air quality was carried out in Shanghai in winter of 2012. The concentrations of NO, NO2, NOx, SO2, CO, and PM2.5increased during haze formation. The average masses of SO4^2-, NO3^-and NH4^＋were 1...A field campaign on air quality was carried out in Shanghai in winter of 2012. The concentrations of NO, NO2, NOx, SO2, CO, and PM2.5increased during haze formation. The average masses of SO4^2-, NO3^-and NH4^＋were 10.3, 11.7 and 6.7 μg/m^3 during the haze episodes, which exceeded the average（9.2, 7.9, and 3.4 μg/m3） of these components in the non-haze days. The mean values for the aerosol scattering coefficient（b sp）, aerosol absorption coefficient（b ap） and single scattering albedo（SSA） were 288.7, 27.7 and0.91 Mm-1, respectively. A bi-peak distribution was observed for the mass concentrations of CO, NO, NO2, and NOx. More sulfate was produced during daytime than that in the evening due to photochemical reactions. The mass concentration of NH4＋achieved a small peak at noontime. NO3-showed lower concentrations in the afternoon and higher concentrations in the early morning. There were obvious bi-peak diurnal patterns for b sp and b ap as well as SSA. b sp and b ap showed a positive correlation with PM2.5mass concentration.（NH4）2SO4, NH4NO3, organic mass, elemental carbon and coarse mass accounted for 21.7%, 19.3%, 31.0%, 9.3% and 12.3% of the total extinction coefficient during non-haze days, and 25.6%, 24.3%, 30.1%, 8.1% and 8.2% during hazy days. Organic matter was the largest contributor to light extinction. The contribution proportions of ammonium sulfate and ammonium nitrate to light extinction were significantly higher during the hazy time than during the non-haze days.展开更多
The diurnal variation of precipitation over the Dabie Mountains(DBM) in eastern China during the 2013 mei-yu season is investigated with forecasts of a regional convection-permitting model. Simulated precipitation is ...The diurnal variation of precipitation over the Dabie Mountains(DBM) in eastern China during the 2013 mei-yu season is investigated with forecasts of a regional convection-permitting model. Simulated precipitation is verified against surface rain-gauge observations. The observed morning precipitation peak on the windward(relative to the prevailing synoptic-scale wind) side of the DBM is reproduced with good spatial and temporal accuracy. The interaction between the DBM and a nocturnal boundary layer low-level jet(BLJ) due to the inertial oscillation mechanism is shown to be responsible for this precipitation peak. The BLJ is aligned with the lower-level southwesterly synoptic-scale flow that carries abundant moisture.The BLJ core is established at around 0200 LST upwind of the mountains. It moves towards the DBM and reaches maximum intensity at about 70 km ahead of the mountains. When the BLJ impinges upon the windward side of the DBM in the early morning, mechanical lifting of moist air leads to condensation and subsequent precipitation.展开更多
An extremely heavy rainfall event lasting from 17 to 22 July 2021 occurred in Henan Province of China, with accumulated precipitation of more than 1000 mm over a 6-day period that exceeded its mean annual precipitatio...An extremely heavy rainfall event lasting from 17 to 22 July 2021 occurred in Henan Province of China, with accumulated precipitation of more than 1000 mm over a 6-day period that exceeded its mean annual precipitation. The present study examines the roles of persistent low-level jets(LLJs) in maintaining the precipitation using surface station observations and reanalysis datasets. The LLJs triggered strong ascending motions and carried moisture mainly from the outflow of Typhoon In-fa(2021). The varying directions of the LLJs well corresponded to the meridional shifts of the rainfall. The precipitation rate reached a maximum during 20-21 July as the LLJs strengthened and expanded vertically into double LLJs, including synoptic-weather-system-related LLJs(SLLJs) at 850–700 hPa and boundary-layer jets(BLJs)at ~950 hPa. The coupling of the SLLJ and BLJ provided strong mid-and low-level convergence on 20 July, whereas the SLLJ produced mid-level divergence at its entrance that coupled with low-level convergence at the terminus of the BLJ on21 July. The formation mechanisms of the two types of LLJs are further examined. The SLLJs and the low-pressure vortex(or inverted trough) varied synchronously as a whole and were affected by the southwestward movement of the WPSH in the rainiest period. The persistent large total pressure gradient force at low levels also maintained the strength of low-level geostrophic winds, thus sustaining the BLJs on the synoptic scale. The results based on a Du-Rotunno 1D model show that the Blackadar and Holton mechanisms jointly governed the BLJ dynamics on the diurnal scale.展开更多
基金supported by the R & D Special Fund for Public Welfare Industry (meteorology)(GYHY201106018)National Key Program for Developing Basic Sciences (Grant No. 2006CB400503)
文摘Based on hourly precipitation data in eastern China in the warm season during 1961-2000,spatial distributions of frequency for 20 mm h 1 and 50 mm h 1 precipitation were analyzed,and the criteria of short-duration rainfall events and severe rainfall events are discussed.Furthermore,the percentile method was used to define local hourly extreme precipitation;based on this,diurnal variations and trends in extreme precipitation were further studied.The results of this study show that,over Yunnan,South China,North China,and Northeast China,the most frequent extreme precipitation events occur most frequently in late afternoon and/or early evening.In the Guizhou Plateau and the Sichuan Basin,the maximum frequency of extreme precipitation events occurs in the late night and/or early morning.And in the western Sichuan Plateau,the maximum frequency occurs in the middle of the night.The frequency of extreme precipitation （based on hourly rainfall measurements） has increased in most parts of eastern China,especially in Northeast China and the middle and lower reaches of the Yangtze River,but precipitation has decreased significantly in North China in the past 50 years.In addition,stations in the Guizhou Plateau and the middle and lower reaches of the Yangtze River exhibit significant increasing trends in hourly precipitation extremes during the nighttime more than during the daytime.
基金National Natural Science Foundation of China (Grant no.91544106)financial support from the Environmental Science Research Institute of Chengdu city for Research of Ozone Formation and Controlling Measures in Chendgu
文摘Chengdu is a megacity in the southwest of China with high ozone(O_3) mixing ratio.Observation of volatile organic compounds(VOCs), NO_2 and O_3 with high temporal resolution was conducted in Chengdu to investigate the chemical processes and causes of high O_3 levels. The hourly mixing ratios of VOCs, NO2, and O_3 were monitored by an online system from 28 August to 7 October, 2016. According to meteorological conditions,Chengdu, with relative warm weather and low wind speed, is favorable to O_3 formation.Part of the O_3 in Chengdu may be transported from the downtown area. In O_3 episodes,the average mixing ratios of NO_2 and O_3 were 20.20 ppbv and 47.95 ppbv, respectively. In non-O_3 episodes, the average mixing ratios of NO_2 and O_3 were 16.38 ppbv and 35.15 ppbv,respectively. The average mixing ratio of total VOCs(TVOCs) was 40.29 ppbv in non-O_3 episodes, which was lower than that in O_3 episodes(53.19 ppbv). Alkenes comprised51.7% of the total O_3 formation potential(OFP) in Chengdu, followed by aromatics which accounted for 24.2%. Ethylene, trans-pentene, propene, and BTEX(benzene, ethylbenzene,toluene, m/p-xylene, o-xylene) were also major contributors to the OFP in Chengdu. In O_3 episodes, intensive secondary formations were observed during the campaign. Oxygenated VOCs(OVOCs), such as acetone, Methylethylketone(MEK), and Methylvinylketone(MVK)were abundant. Isoprene rapidly converted to MVK and Methacrolein(MACR) during O_3 episodes. Acetone was mainly the oxidant of C3-C5 hydrocarbons.
基金supported by grants from the National Basic Key Research Program (973) under Grant No. 2006CB403606the National Key Technology R&D Program under Grant No. 2007BAC29B04the National Science Foundation Project for Post-doctoral Scientists of China under Grant No. 20080440343
文摘The present study examined the diurnal variations of summer precipitation in the Beijing area by usingsubdaily precipitation and wind observations. A combined effect of topography and urbanization on thecharacteristics of diurnal variations was suggested. It was shown that stations located in the plain areaexhibited typical night rain peaks, whereas those in the mountainous area exhibited clear afternoon peaks ofprecipitation diurnal variations. The precipitation peaks were associated with wind fields around the Beijingarea, which were found to be highly modulated by mountain-valley circulation and urban-country circulation.The lower-tropospheric wind exhibited a clear diurnal shift in its direction from north at 0800 LST to southat 2000 LST, which reflected mountain-valley circulation. The transitions from valley to mountain windand the opposite generally happened after sunset and sunrise, respectively, and both occurred earlier for thestations located closer to mountains. By comparing the diurnal variations of precipitation at stations in anortheast suburb, an urban area, and a southwest suburb, it was revealed that the northeast suburb grouphad the highest normalized rainfall frequency, but the southwest group had the lowest from late afternoon tolate evening. On the contrary, in the early morning from about 0200 to 1000 LST, the southwest group andurban group had the highest normalized rainfall frequency. This pattern might originate from the combinedeffects of mountain-valley topography and urbanization.
基金Supported by the China Meteorological Administration Special Public Welfare Research Fund (GYHY201206004,GYHY201206003,and GYHY200906003)National (Key) Basic Research and Development (973) Program of China (2013CB430106)
文摘Short-duration heavy rainfall（SDHR） is a type of severe convective weather that often leads to substantial losses of property and life. We derive the spatiotemporal distribution and diurnal variation of SDHR over China during the warm season（April–September） from quality-controlled hourly raingauge data taken at 876 stations for 19 yr（1991–2009）, in comparison with the diurnal features of the mesoscale convective systems（MCSs） derived from satellite data. The results are as follows. 1） Spatial distributions of the frequency of SDHR events with hourly rainfall greater than 10–40 mm are very similar to the distribution of heavy rainfall（daily rainfall 50 mm） over China's Mainland. 2） SDHR occurs most frequently in South China such as southern Yunnan, Guizhou, and Jiangxi provinces, the Sichuan basin, and the lower reaches of the Yangtze River, among others. Some SDHR events with hourly rainfall 50 mm also occur in northern China, e.g., the western Xinjiang and central-eastern Inner Mongolia. The heaviest hourly rainfall is observed over the Hainan Island with the amount reaching over 180 mm. 3） The frequency of the SDHR events is the highest in July, followed by August. Analysis of pentad variations in SDHR reveals that SDHR events are intermittent, with the fourth pentad of July the most active. The frequency of SDHR over China's Mainland increases slowly with the advent of the East Asian summer monsoon, but decreases rapidly with its withdrawal. 4） The diurnal peak of the SDHR activity occurs in the later afternoon（1600–1700 Beijing Time（BT））, and the secondary peak occurs after midnight（0100–0200 BT） and in the early morning（0700–0800 BT）; whereas the diurnal minimum occurs around late morning till noon（1000–1300 BT）. 5） The diurnal variation of SDHR exhibits generally consistent features with that of the MCSs in China, but the active periods and propagation of SDHR and MCSs difer in diferent regions. The number and duration of local maxima in the d
基金Project supported by the National Basic Research Program (973) of China (No. 2007CB407300)the National Natural Science Foundation of China (No. 40675074)+1 种基金the Pilot Project of Knowledge Innovation Program of Chinese Academy of Sciences (No. KZCX3-SW-231)a grant from the SKLLQG, Chinese Academy of Sciences and the Research Grants Council of Hong Kong (No. PolyU5145/03E, PolyU5197/05E).
文摘An intensive observation of organic carbon （OC） and element carbon （EC） in PM10 and gaseous materials （SO2, CO, and O3,） was conducted continuously to assess the characteristics of wintertime carbonaceous aerosols in an urban area of Beijing, China. Results showed that the averaged total carbon （TC） and PM10 concentrations in observation period are 30.2±120.4 and 172.6±198.3 μ/m^3 respectively. Average OC concentration in nighttime （24.9±19.6 μ/m^3 was 40% higher than that in daytime （17.7±10.9 μ/m^3. Average EC concentrations in daytime （8.8±15.2 μ/m^3 was close to that in nighttime （8.9±15.1 μ/m^3. The OC/EC ratios in nighttime ranging from 2.4 to 2.7 are higher than that in daytime ranging from 1.9 to 2.0. The concentrations of OC, EC, PM10 were low with strong winds and high with weak winds. The OC and EC were well correlated with PM10, CO and SO2, which implies they have similar sources. OC and EC were not well correlated with O3. By considering variation of OC/EC ratios in daytime and night time, correlations between OC and O3, and meteorological condition, we speculated that OC and EC in Beijing PM10 were emitted as the primary particulate form. Emission of motor vehicle with low OC/EC ratio and coal combustion sources with high OC/EC ratio are probably the dominant sources for carbonaceous aerosols in Beijing in winter. A simple method was used to estimate the relative contribution of sources to carbonaceous aerosols in Beijing PM10. Motor vehicle source accounts for 80% and 68%, while coal combustion accounts for 20% and 32% in daytime and nighttime, respectively in Beijing. Averagely, the motor vehicle and coal combustion accounted for 74% and 26%, respectively, for carbonaceous aerosols during the observation period. It points to the motor vehicle is dominant emission for carbonaceous aerosols in Beijing PM10 in winter period, which should be paid attention to control high level of PM10 in Beijing effectively.
基金Project supported by the National Basic Research Project(973)of China(No.2005CB422203)the National Post-Doctor Foundation of China(No.20060390990).
文摘The aerosol number concentration and size distribution were measured with the newly developed Wide-range Particle Spectrometer in summer and winter of 2006 at the urban site of Jinan City. Here reported the characteristics of fine particles of the different observation seasons. Relative high number concentrations for the particles in the diameter range of 10-500 nm were observed in both seasons. It was found that the dominant number distributed in particle diameter smaller than 100 nm and the percentage over the number concentration of all air particles is much higher than what has been measured in other urban sites over the world. The number mean diameter in summer was much smaller than in winter, strongly suggesting the different origin of ultrafine particles in different seasons. That is, particles in ultrafine mode mainly came from nucleation and new particle formation in summer while from traffic emission in winter. The diurnal variation also supported this point. Number concentration in the diameter range of 10-200 um got their peak values at noontime, well correlated with the mixing ratio of SO2 and the intensity of solar radiation in summer. While in winter, those in the same diameter range showed the main peaks during the traffic hours happened in the morning and evening.
基金jointly sponsored by a project of the State Key Laboratory of Severe Weather,Chinese Academy of Meteorological Sciences(Grant No.2011LASWA15)the National Key Basic Research and Development Project of China(Grant No.2012CB417201)the National Natural Science Foundation of China(Grant No.40930951)
文摘Diurnal variations of two mountain-plain solenoid （MPS） circulations associated with ＂first-step＂ terrain [Tibetan Plateau （TP）] and ＂second-step＂ terrain （high mountains between the TP and ＂east plains＂） in China and their influence on the south west vortex （SWV） and the mei-yu front vortex （MYFV） were investigated via a semi-idealized mesoscale numerical model [Weather Research and Forecasting （WRF）] simulation integrated with ten-day average fields （mei-yu period of 1-10 July 2007）. The simulations successfully reproduced two MPS circulations related to first and second-step terrain, diurnal vari- ations from the eastern edge of the TP to the Yangtze River-Huaihe River valleys （YHRV）, and two precipitation maximum centers related to the SWV, MYFV. Analyses of the averaged final seven-day simulation showed the different diurnal peaks of precipitation at different regions： from the aftemoon to early evening at the eastern edge of the TP; in the early evening to the next early morning in the Sichuan Basin （SCB）; and in the late evening to the next early morning over the mei-yu front （MYF）. Analyses of individual two-day cases confirmed that the upward branches of the nightlime MPS circulations enhanced the precipitation over the SWV and the MYFV and revealed that the eastward extension of the SWV and its con vection were conducive to triggering the MYFVs. The eastward propagation of a rainfall streak from the eastern edge of the TP to the eastern coastal region was primarily due to a series of convective activities of several systems from west to east, including the MPS between the TP and SCB, the SWV, the MPS between second-step terrain and tile east plains, and the MYFV.
基金supported by Knowledge Innovation Program of the Chinese Academy of Sciences (Grant No.KZCX2-YW- Q11-04)National Basic Research Program of China (Grant Nos.2011CB403505 and 2010CB950402)National Natural Science Foundation of China (Grant Nos.40975052)
文摘Climatological characteristics of diurnal variations in summer precipitation over the Asian monsoon region are comprehensively investigated based on the Tropical Rainfall Measuring Mission(TRMM) satellite data during 1998-2008.The topographic influence on the diurnal variations and phase propagations of maximum precipitation are identified according to spatiotemporal distributions of the amplitude and peak time of the diurnal precipitation.The amplitude and phase of diurnal precipitation show a distinct geographical pattern.Significant diurnal variations occur over most of continental and coastal areas including the Maritime Continent,with the relative amplitude exceeding 40%,indicating that the precipitation peak is 1.4 times the 24-h mean.Over the landside coasts such as southeastern China and Indochina Peninsula,the relative amplitude is even greater than 100%.Although the diurnal variations of summer precipitation over the continental areas are characterized by an afternoon peak(1500-1800 Local Solar Time(LST)),over the central Indochina Peninsula and central and southern Indian Peninsula the diurnal phase is delayed to after 2100 LST,suggesting the diurnal behaviors over these areas different from the general continental areas.The weak diurnal variations with relative amplitudes less than 40% exist mainly over oceanic areas in the western Pacific and most of Indian Ocean,with the rainfall peak mainly occurring from midnight to early morning(0000-0600 LST),indicating a typical oceanic regime characterized by an early morning peak.However,apparent exceptions occur over the South China Sea(SCS),Bay of Bengal(BOB),and eastern Arabian Sea,with the rainfall peak occurring in daytime(0900-1500 LST).Prominent meridional propagations of the diurnal phase exist in South Asia and East Asia.Along the eastern Indian Peninsula,there is not only the southward phase propagation with the peak occurring around 25°N but also the northward phase propagation with the peak beginning with the southernmost continent,and both reach
基金supported by the National Key Research and Development Program of China (Grant No. 2016YFA0600704)the National Natural Science Foundation of China (Grant No. 41575068 and 41530530)
文摘The mountain-plains solenoid(MPS) and boundary-layer inertial oscillation(BLO) are two typical regional forcings at the diurnal time scale. Their relative role in regulating the diurnal variations of summer rainfall over North China and their change under different monsoon conditions are studied using a 19-yr archive of satellite rainfall and reanalysis data. It is shown that both a strong MPS and BLO can increase nocturnal rainfall in the North China plains but exhibit evident regional differences. The MPS-induced nocturnal rainfall is relatively confined to the plains adjacent to mountains from late night to morning, due to the upward branch of the nighttime MPS. In contrast, the BLO-induced nocturnal rainfall strengthens from early evening and is more extensive in early morning over the open plains further east. The contrasting effect in the evening is related to the convergent(divergent) easterly anomaly in the plains under the BLO(MPS). The BLO also induces the relatively strong enhancement of moisture convergence and high humidity by the southerly anomaly at late night. On strong monsoon days, the nocturnal rainfall amount associated with the MPS and BLO increases considerably in the plains.Both regional forcings become effective in regulating the rainfall diurnal cycle with enhanced moisture convergence under monsoon conditions. Their induced diurnal amplitudes of moisture convergence can be comparable to the daily mean by monsoon flow. The regional forcings thus couple with monsoon flow to strengthen rainfall in the plains, particularly from late night to morning. The results highlight that a combination of regional and large-scale forcings can strongly regulate the warm-season climate.
基金The Key Program of Knowledge Innovation Project of Chinese Academy of Sciences under contract No.KZCX1-YW-12the National 863 Program under contract Nos 2008AA09A401 and 2006AA09A109
文摘Based on in-situ time series data from the acoustic Doppler current profiler （ADCP） and thermistor chain in Wenchang area, a sequence of internal solitary wave （ISW） packets was observed in September 2005, propagating northwest on the continental shelf of the northwestern South China Sea （SCS）. Corresponding to different stratification of the water column and tidal condition, both elevation and depression ISWs were observed at the same mooring location with amplitude of 35 m and 25 m respectively in different days. Regular arrival of the remarkable ISW packets at approximately the diurnal tidal period and the dominance of diurnal internal waves in the study area, strongly suggest that the main energy source of the waves is the diurnal tide. Notice that the wave packets were all riding on the troughs and shoulders of the internal tides, they were probably generated locally from the shelf break by the evolution of the internal tides due to nonlinear and dispersive effects.
基金supported by the Major National Basic Research Program of China (973 Program) on Global Change (Grant No.2010CB951902)the National Natural Science Foundation of China (Grant Nos. 40625014,40705025,40921003,and 41005044)
文摘In this study, records from a 3-yr intensified observational experiment at eight stations along the hillside of Seqilashan over the southeastern Tibetan Plateau were analyzed and combined with records at 28 routine observation stations in the Chinese National Meteorological Station Network to investigate the influences of station location on the different diurnal rainfall variations between station records and Tropical Rainfall Measuring Mission （TRMM） data products. The results indicate that the diurnal variation of warm season rainfall is closely related to location of stations. The prevailing nocturnal rainfall peak in observations at routine stations can be largely attributed to the relatively lower location of the stations, which are mostly situated in valleys. The records at Seqilashan stations on hillsides revealed an evident diurnal afternoon peak of warm season rainfall, similar to that indicated by TRMM data. The different diurnal phases between valley and hillside stations are closely related to the orographically induced regional circulations caused by the complex topography over the Tibetan Plateau. The results of this study indicate that the prevailing nocturnal rainfall associated with the relatively lower location of routine observation stations can partially explain the diurnal rainfall variations between observation station records and TRMM data.
基金National Natural Science Foundation of China, No.20777073 Acknowledgements The authors would like to thank Sun Pu of Anhui Hydrological Bureau for the help of sampling in the field.
文摘This study was performed at three eutrophic rivers in Southeast China aiming to determine the magnitude and patterns of dissolved N2O concentrations and fluxes over a seasonal （in 2009） and diurnal （24 h） temporal scale.The results showed that N2O concentrations varied from 0.28 to 0.38 （mean 0.32±0.04）,0.29 to 0.46 （mean 0.37±0.07）,and 2.07 to 3.47 （mean 2.84±0.63） μg N-N2O L-1 in the Fengle,Hangbu and Nanfei rivers,respectively,in the diurnal study performed during the summer of 2008.The study found that mean N2O concentration and estimated N2O flux （67.89 ± 6.71 μg N-N2O m-2 h-1） measured from the Nanfei River with serious urban wastewater pollution was significantly higher than those from the Fengle and the Hangbu Rivers with agricultural runoff.In addition,the seasonal study during June and December of 2009 also showed that the mean N2O concentration （10.59±14.67 μg N-N2O L-1） and flux （236.87±449.74 μg N-N2O m-2 h-1） observed from the Nanfei River were significantly higher than those from the other two rivers.Our study demonstrated both N2O concentrations and fluxes exhibited seasonal and diurnal fluctuations.Over three consecutive days during the summer of 2008,N2O accumulation rates varied within the range of 3.91-7.21,2.76-15.71,and 3.23-30.03 μg N-N2O m-2 h-1 for the Fengle,Hangbu and Nanfei Rivers,respectively,and exponentially decreased with time.
基金National Natural Science Foundation of China, No.41461003 National Basic Research Program of China （973 Program）, No.2013CBA01801
文摘To investigate the diurnal variation of summer precipitation in the Qilian Mountains in the northeast Tibetan Plateau, the hourly precipitation amount for this region during the summers of 2008-2014 are analyzed using an hourly merged precipitation product at 0.1°×0.1 ° resolution. The main results are as follows. （1） The spatial distribution and temporal variation of mean hourly precipitation amount and frequency are generally similar and hourly precipitations in the eastern and middle portions are larger and more frequent than that in the western portion. The high value area of precipitation intensity is obviously different from that of precipitation amount and frequency. （2） The spatial distribution of daytime precipitation is generally similar to that of nighttime precipitation, and the daytime precipitation is heavier than the nighttime precipitation. （3） The change rate of precipitation has a maximum at 20：00 Beijing time, and a minimum at 12：00. The hourly precipitation amount significantly correlated with frequency, especially for the middle and eastern portions.
基金supported by the Ministry of Science and Technology of China (No. 2013CB955804)the National Natural Science Foundation of China (Nos. 41175018, 41475113)the Ministry of Environmental Protection of China (Nos. 201209001, 201409008, 201209007)
文摘A field campaign on air quality was carried out in Shanghai in winter of 2012. The concentrations of NO, NO2, NOx, SO2, CO, and PM2.5increased during haze formation. The average masses of SO4^2-, NO3^-and NH4^＋were 10.3, 11.7 and 6.7 μg/m^3 during the haze episodes, which exceeded the average（9.2, 7.9, and 3.4 μg/m3） of these components in the non-haze days. The mean values for the aerosol scattering coefficient（b sp）, aerosol absorption coefficient（b ap） and single scattering albedo（SSA） were 288.7, 27.7 and0.91 Mm-1, respectively. A bi-peak distribution was observed for the mass concentrations of CO, NO, NO2, and NOx. More sulfate was produced during daytime than that in the evening due to photochemical reactions. The mass concentration of NH4＋achieved a small peak at noontime. NO3-showed lower concentrations in the afternoon and higher concentrations in the early morning. There were obvious bi-peak diurnal patterns for b sp and b ap as well as SSA. b sp and b ap showed a positive correlation with PM2.5mass concentration.（NH4）2SO4, NH4NO3, organic mass, elemental carbon and coarse mass accounted for 21.7%, 19.3%, 31.0%, 9.3% and 12.3% of the total extinction coefficient during non-haze days, and 25.6%, 24.3%, 30.1%, 8.1% and 8.2% during hazy days. Organic matter was the largest contributor to light extinction. The contribution proportions of ammonium sulfate and ammonium nitrate to light extinction were significantly higher during the hazy time than during the non-haze days.
基金supported by the Special Foundation of the China Meteorological Administration (Grant No.GYHY201506006)supported by the National Science Foundation of China (Grant Nos.41405100,41322032 and 41275031)
文摘The diurnal variation of precipitation over the Dabie Mountains(DBM) in eastern China during the 2013 mei-yu season is investigated with forecasts of a regional convection-permitting model. Simulated precipitation is verified against surface rain-gauge observations. The observed morning precipitation peak on the windward(relative to the prevailing synoptic-scale wind) side of the DBM is reproduced with good spatial and temporal accuracy. The interaction between the DBM and a nocturnal boundary layer low-level jet(BLJ) due to the inertial oscillation mechanism is shown to be responsible for this precipitation peak. The BLJ is aligned with the lower-level southwesterly synoptic-scale flow that carries abundant moisture.The BLJ core is established at around 0200 LST upwind of the mountains. It moves towards the DBM and reaches maximum intensity at about 70 km ahead of the mountains. When the BLJ impinges upon the windward side of the DBM in the early morning, mechanical lifting of moist air leads to condensation and subsequent precipitation.
基金supported by Guangdong Major Project of Basic and Applied Basic Research(2020B0301030004)the National Natural Science Foundation of China(Grant Nos.42122033,41875055,and 42075006)Guangzhou Science and Technology Plan Projects(202002030346 and 202002030196).
文摘An extremely heavy rainfall event lasting from 17 to 22 July 2021 occurred in Henan Province of China, with accumulated precipitation of more than 1000 mm over a 6-day period that exceeded its mean annual precipitation. The present study examines the roles of persistent low-level jets(LLJs) in maintaining the precipitation using surface station observations and reanalysis datasets. The LLJs triggered strong ascending motions and carried moisture mainly from the outflow of Typhoon In-fa(2021). The varying directions of the LLJs well corresponded to the meridional shifts of the rainfall. The precipitation rate reached a maximum during 20-21 July as the LLJs strengthened and expanded vertically into double LLJs, including synoptic-weather-system-related LLJs(SLLJs) at 850–700 hPa and boundary-layer jets(BLJs)at ~950 hPa. The coupling of the SLLJ and BLJ provided strong mid-and low-level convergence on 20 July, whereas the SLLJ produced mid-level divergence at its entrance that coupled with low-level convergence at the terminus of the BLJ on21 July. The formation mechanisms of the two types of LLJs are further examined. The SLLJs and the low-pressure vortex(or inverted trough) varied synchronously as a whole and were affected by the southwestward movement of the WPSH in the rainiest period. The persistent large total pressure gradient force at low levels also maintained the strength of low-level geostrophic winds, thus sustaining the BLJs on the synoptic scale. The results based on a Du-Rotunno 1D model show that the Blackadar and Holton mechanisms jointly governed the BLJ dynamics on the diurnal scale.
